Ionic liquid-derived charged polymers to show highly thermoresponsive LCST-type transition with water at desired temperatures.

نویسندگان

  • Yuki Kohno
  • Yuki Deguchi
  • Hiroyuki Ohno
چکیده

A polymerised ionic liquid (poly(IL)) having suitable hydrophobicity undergoes a strongly temperature-sensitive LCST-type phase transition with pure water and also with aqueous salt solution, and the resulting hydrated poly(IL) further undergoes a sharp and reversible liquid-to-gel transition at ambient temperatures.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Toward the dynamic phase transition mechanism of a thermoresponsive ionic liquid in the presence of different thermoresponsive polymers.

The influence of two thermoresponsive polymers, poly(N-isopropylacrylamide) (PNIPAM) and poly(N-vinylcaprolactam) (PVCL), on the phase transition behavior of a thermoresponsive ionic liquid, tributylhexylphosphonium 3-sulfopropylmethacrylate ([P4,4,4,6][MC3S]), was investigated. An obvious distinction was observed in the LCSTs and morphologies of [P4,4,4,6][MC3S]-PNIPAM and [P4,4,4,6][MC3S]-PVC...

متن کامل

Reversible water uptake/release by thermoresponsive polyelectrolyte hydrogels derived from ionic liquids.

Thermoresponsive polyelectrolyte hydrogels, derived from tetra-n-alkylphosphonium 3-sulfopropyl methacrylate-type ionic liquid monomers, show reversible water uptake/release, in which the gels absorb/desorb water for at least ten cycles via a lower critical solution temperature-type phase transition.

متن کامل

LCST-type polymers based on chiral-polymeric ionic liquids.

The self-assembly of linear polymers containing chiral IL units generates a high-order supramacromolecular structure with a complex hierarchical architecture, which is able to exhibit thermoresponsive behavior (lower critical solution temperature: LCST) with different structural elements that can be used to fine tune this LCST.

متن کامل

Thermoresponsive PNIPAAM bottlebrush polymers with tailored side-chain length and end-group structure.

We explore the phase behaviour, solution conformation, and interfacial properties of bottlebrush polymers with side-chains comprised of poly(N-isopropylacrylamide) (PNIPAAM), a thermally responsive polymer that exhibits a lower critical solution temperature (LCST) in water. PNIPAAM bottlebrush polymers with controlled side-chain length and side-chain end-group structure are prepared using a "gr...

متن کامل

Thermoresponsive poly(N-vinylcaprolactam) as stationary phase for aqueous and green liquid chromatography

Poly(N-vinylcaprolactam) (PVCL) connected to aminopropyl silica is a new stationary phase for temperature responsive liquid chromatography (TR-LC). PVCL shows a transition from hydrophilic to hydrophobic interaction between 30 and 40°C. The synthesis is described in detail. The temperature responsive characteristic of the phase is illustrated with a mixture of steroids using pure water as mobil...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Chemical communications

دوره 48 97  شماره 

صفحات  -

تاریخ انتشار 2012